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Proton diffusion pathways and rates in Y-doped BaZrO(3) solid oxide electrolyte from quantum mechanics

We carried out quantum mechanical calculations (Perdew-Becke-Ernzerhof flavor of density functional theory) on 12.5% Y-doped BaZrO(3) (BYZ) periodic structures to obtain energy barriers for intraoctahedral and interoctahedral proton transfers. We find activation energy (E(a)) values of 0.48 and 0.49...

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Detalhes bibliográficos
Main Authors: Merinov, Boris, Goddard, William
Formato: Artigo
Idioma:Inglês
Publicado em: American Institute of Physics 2009
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2832051/
https://ncbi.nlm.nih.gov/pubmed/19466855
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1063/1.3122984
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