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The structure of the biliverdin radical intermediate in phycocyanobilin:ferredoxin oxidoreductase identified by high-field EPR and DFT

The cyanobacterial enzyme phycocyanobilin:ferredoxin oxidoreductase (PcyA) catalyzes the two-step four-electron reduction of biliverdin IXα to phycocyanobilin, the precursor of biliprotein chromophores found in phycobilisomes. It is known that catalysis proceeds via paramagnetic radical intermediate...

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Detalhes bibliográficos
Main Authors: Stoll, Stefan, Gunn, Alexander, Brynda, Marcin, Sughrue, Wesley, Kohler, Amanda C., Ozarowski, Andrew, Fisher, Andrew J., Lagarias, J. Clark, Britt, R. David
Formato: Artigo
Idioma:Inglês
Publicado em: 2009
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Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2753389/
https://ncbi.nlm.nih.gov/pubmed/19159240
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja808573f
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