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Synthetic Studies on Et-743. Assembly of the Pentacyclic Core and a Formal Total Synthesis

A formal total synthesis of the potent anticancer agent Et-743 is described. The tetrahydroisoquinoline core is stereoselectively constructed using a novel radical cyclization of a glyoxalimine. Further elaboration of this core rapidly accessed the pentacyclic core of Et-743, but a mixture of regios...

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Detalhes bibliográficos
Main Authors: Fishlock, Dan, Williams, Robert M.
Formato: Artigo
Idioma:Inglês
Publicado em: 2008
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2736329/
https://ncbi.nlm.nih.gov/pubmed/18687003
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo801159k
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