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VTVH-MCD and DFT Studies of Thiolate Bonding to {FeNO}(7)/{FeO(2)}(8) Complexes of Isopenicillin N synthase: Substrate Determination of Oxidase versus Oxygenase Activity in Non-Heme Fe Enzymes
Isopenicillin N synthase (IPNS) is a unique mononuclear non-heme Fe enzyme that catalyzes the four electron oxidative double ring closure of its substrate ACV. A combination of spectroscopic techniques including EPR, absorbance, circular dichroism (CD), magnetic CD, and variable-temperature, variabl...
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| Main Authors: | , , , , |
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| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2007
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2536647/ https://ncbi.nlm.nih.gov/pubmed/17506560 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja071364v |
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