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Relation between the Widom line and the breakdown of the Stokes–Einstein relation in supercooled water

Supercooled water exhibits a breakdown of the Stokes–Einstein relation between the diffusion constant D and the alpha relaxation time τ(α). For water simulated with two different potentials, TIP5P and ST2, we find that the temperature of the decoupling of diffusion and alpha relaxation correlates wi...

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Detalhes bibliográficos
Principais autores: Kumar, Pradeep, Buldyrev, S. V., Becker, S. R., Poole, P. H., Starr, F. W., Stanley, H. E.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2007
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC1887548/
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0702608104
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