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Ambiphilic Frustrated Lewis Pair Exhibiting High Robustness and Reversible Water Activation: Towards the Metal-Free Hydrogenation of Carbon Dioxide

The synthesis and structural characterization of a phenylene-bridged Frustrated Lewis Pair (FLP) having a 2,2,6,6‑tetramethylpiperidine (TMP) as the Lewis base and a 9-borabicyclo[3.3.1]nonane (BBN) as the Lewis acid is reported. This FLP exhibits unique robustness towards the products of carbon dio...

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Principais autores: Étienne Rochette, Marc-André Courtemanche, Alexander P. Pulis, Wenhua Bi, Frédéric-Georges Fontaine
Formato: Artigo
Idioma:Inglês
Publicado: MDPI AG 2015-06-01
Series:Molecules
Assuntos:
carbon dioxide
Frustrated Lewis Pairs
hydrogenation
Lewis acid
ambiphilic molecules
catalysis
Acceso en liña:http://www.mdpi.com/1420-3049/20/7/11902
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