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Ligand Modification Transforms a Catalase Mimic into a Water Oxidation Catalyst()
The catalytic reactivity of the high-spin Mn(II) pyridinophane complexes [(Py(2)NR(2))Mn(H(2)O)(2)](2+) (R = H, Me, tBu) towards O(2) formation is reported. With small macrocycle N-substituents (R = H, Me), the complexes catalytically disproportionate H(2)O(2) in aqueous solution. While this catalys...
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| Main Authors: | , , , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2014
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4167389/ https://ncbi.nlm.nih.gov/pubmed/25044487 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201402407 |
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