Monitoring molecular dynamics using coherent electrons from high harmonic generation

We report a previously undescribed spectroscopic probe that makes use of electrons rescattered during the process of high-order harmonic generation. We excite coherent vibrations in SF(6) using impulsive stimulated Raman scattering with a short laser pulse. A second, more intense laser pulse generat...

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Bibliografiske detaljer
Main Authors: Wagner, Nicholas L., Wüest, Andrea, Christov, Ivan P., Popmintchev, Tenio, Zhou, Xibin, Murnane, Margaret M., Kapteyn, Henry C.
Format: Artigo
Sprog:Inglês
Udgivet: National Academy of Sciences 2006
Fag:
Physical Sciences
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC1533881/
https://ncbi.nlm.nih.gov/pubmed/16895984
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0605178103
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